Target: Captain Black!

Francis Matthews Captain Scarlet (voice)

Ed Bishop Captain Blue (voice)

Donald Gray Colonel White / Captain Black / The Mysterons (voice)

Cy Grant Lieutenant Green (voice)

Elizabeth Morgan Destiny Angel (voice)

Jeremy Wilkin Captain Ochre / Andre Verdain / Major Gravener (voice)

Gary Files Captain Magenta / Doig / Sergeant (voice)

Paul Maxwell Captain Grey / Guard (voice)

Janna Hill Symphony Angel (voice)

David Healy Kruger / Geiger Operator / Dr. Mitchell (voice)

Sylvia Anderson Gabrielle (voice)

Charles Tingwell Harris (voice)

Martin King Richards / Garage Mechanic / Security Chief / Carl / Guard / Dr. Baxter (voice)